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博士生霍存宝参加国际会议回国报告

发布时间:2023-07-10 点击数:

汇报时间2023711(星期三) 上午10: 00

汇报地点:曲江校区南一楼A3楼会议室

汇报人:霍存宝

国际会议信息

会议名称:The XVIIIth Conference of the European Ceramic Society (XVIII ECERS)

会议时间:July 2-6, 2023

会议地点:LYON CONVENTION CENTRE, Lyon, France.

会议简介:The XVIIIth Conference of the European Ceramic Society will take place in Lyon, on 2-6 July 2023. Lyon, where the Rhône and the Saône rivers meet, has always been a city of exchanges and industrial development, with major historic landmarks. ‘Lugdunum’ was founded in 43BC by the Romans and served as the capital of Gaul. It was also famous, as the world capital of silk, during the French Renaissance. Lyon’s cuisine is famous all over the world, the cinema was invented by the Lumière brothers in this City of Lights, surrounded by prestigious wine areas where you can taste Beaujolais, Burgundy and Côtes-du-Rhône, not far from the Alps and of course Mont Blanc. Lyon is also the city of cutting edge industry and engineering, especially in the fields of chemistry and materials, bio-technology and medicine, mobility systems, with numerous schools and faculties created to answer technological and societal needs. Thus, it is a great pleasure to welcome ceramists in the City of Lights, to share the latest discoveries in ceramic science and technology, reconnect with colleagues from around the world, in a convivial conference atmosphere . The conference, hosting ceramic experts from industry and academia, offering a unique opportunity to participate in an international event covering the development and applications of ceramic-based systems. In addition to the now traditional symposia dealing with innovative processing, thermo-mechanical properties, modelling and ceramics for different high-tech applications, emphasis will also be given to advanced characterization techniques, silicate-based ceramics and materials for building applications, as well as the place of ceramics in necessary sustainable development. Lyon has been growing and evolving for 2,000 years: it is today a leading sustainable destination. Therefore, intent on reducing our environmental impact, we will make this XVIIIth ECerS conference a truly “think green” event.

参会论文信息

Title: 3D Printing of Hierarchically Porous Monolithic TS‐1 Catalyst for One-Pot Synthesis of Ethylene Glycol

Author: Cunbao Huo, Xiaoyong Tian, Zhengping Qiu, Tengfei Liu, Lingling Wu

Abstract: Structured monolithic catalysts have attracted increasing attention in the petrochemical industry due to their advantages of high heat and mass transfer rate, easy scale-up, and reusability. Herein, we put forward a strategy for one-step preparation of SiO2-based monolithic TS-1 catalysts with optimal hierarchical scaffolds by combining the flow field simulation of the reactor and 3D printing technology. Tunable hierarchical porosity from nano to micro scales, suitable pore characteristics, and numerous active sites have been obtained by innovatively combining the spherical porous structure of TS-1/SiO2 material, direct ink writing (DIW) and post-sintering processes. Combined with computational fluid dynamics (CFD) analysis, the effects of different channel offset angles, axial and radial channel sizes on the 3D printed monolithic TS-1 in the catalytic reaction of one-step oxidation of ethylene to ethylene glycol (EG) were verified. 3D-printed monolithic TS-1 catalysts exhibited superior crush strengths (135.11 N/cm) and extraordinary catalytic efficiency, in which the yield of EG reached 82.7%, and the utilization of hydrogen peroxide reached 85.3%. Moreover, the 3D printed TS-1 monolith maintained high catalytic performance over 5 reusable cycles, which solved the problem that traditional catalysts are difficult to be manufactured, separated, and recycled, and presented considerable prospects in reactions requiring fluid agitation.


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